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Sharan and Sitak lost to the Brazilian-Croat pair 6-7 3-6 in a second-round match that lasted one hour and 17 minutes.
With Sharan’s loss, India’s campaign in the men’s doubles ended as Rohan Bopanna had made a first-round exit on Wednesday.
On Thursday, comeback star Sania Mirza’s first Grand Slam outing after maternity leave also ended with an early exit as the Indian ace retired mid-way into her women’s doubles first-round match due to a calf injury.
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Bopanna is the only Indian left in the fray now. The 39-year-old will partner Ukraine’s Nadiia Kichenok in the mixed doubles event.
The duo will take on France’s Nicolas Mahut and Zhang Shai of China in the first round on Saturday.