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He was 74.
His end came at 2.35 am at a private hospital in Parumala in Pathanamthitta district while undergoing treatment for post-COVID-19 complications, he said.
The senior priest, who had been suffering from lung cancer since December 2019, had recovered from the COVID-19 infection in February this year.
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He was enthroned as the Catholicos of the East & Malankara Metropolitan in November 2010.