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Concerns over rising inflation and foreign fund outflows in the wake of the uncertain geopolitical situation also sapped investor confidence.
In a highly volatile trade, the Sensex finished 703.59 points or 1.23 percent lower at 56,463.15 as fag-end selling emerged. In choppy trade, the benchmark hit a high of 57,464.08 and a low of 56,009.07 during the day.
The NSE Nifty declined 215 points or 1.25 per cent to settle at 16,958.65.
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From the 30-share Sensex pack, HDFC, HDFC Bank, Infosys, ITC, Tech Mahindra and HCL Technologies were among the major laggards.
In contrast, Reliance Industries, ICICI Bank, State Bank of India, and Bajaj Finance were the gainers.
In Asia, markets in Shanghai and Hong Kong settled lower, while Seoul and Tokyo were up.
Markets in Europe were also trading lower in the afternoon session.
Stocks in the US had ended marginally lower on Monday.
International oil benchmark Brent crude declined 1.39 percent to USD 111.6 per barrel.
Foreign institutional investors continued their selling spree, offloading shares worth a net Rs 6,387.45 crore on Monday, according to exchange data.